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EUBCE 2026 - Thomas MÜLLER - From Lignin to Polyols: Combined Catalytic and Electrochemical Approach for Advanced Biomass Conversion

From Lignin to Polyols: Combined Catalytic and Electrochemical Approach for Advanced Biomass Conversion

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Biomass conversion into bio-based chemicals and high-value compounds (part 2)

From Lignin to Polyols: Combined Catalytic and Electrochemical Approach for Advanced Biomass Conversion

Short Introductive summary

Lignin represents the largest renewable source of aromatic carbon, yet its structural heterogeneity limits its integration into chemical value chains. This work presents a combined catalytic–electrochemical approach for converting diverse technical lignins into tunable oligomers and bio-based polyols suitable for polyurethane applications. Controlled catalytic depolymerization (hydrogenolysis and oxidation) generates low-molecular-weight substrates enriched in ß–O–4 cleavage products, which are subsequently upgraded in mild electrochemical processes using RuO2 and Cu-based electrodes. These promote selective a-functionalization, ß–O–4 scission, and aldehyde-to-alcohol reduction, achieving faradaic efficiencies above 60%. Comprehensive NMR analysis reveals hydroxyl-rich oligomeric products with functional-group distributions aligned with polyol requirements. The integrated workflow offers a scalable and energy-efficient route to renewable aromatic intermediates, addressing key challenges in lignin valorization and supporting the transition toward circular, bio-based polymer feedstocks.

Presenter

Moderator portrait

Thomas MÜLLER

Ruhr-Universität Bochum, Faculty of Mechanical Engineering, GERMANY

Presenter's biography

Prof. T.E. Müller holds the chair Carbon Sources and Conversion at Ruhr-Universität Bochum, where he develops new chemical processes at the interface of the chemical industry and the energy sector. His work centres on renewable feedstocks, CO2 utilisation, and sustainable chemical technologies.

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Co-authors:

T.E. Müller, Ruhr-Universität Bochum, GERMANY
E. Sabri, Ruhr-Universität Bochum, GERMANY
G.P. Sorrentino, Ruhr-Universität Bochum, GERMANY
O. Tabot, Ruhr-Universität Bochum, GERMANY
U. Apfel, Ruhr-Universität Bochum, GERMANY
R. Stoll, Ruhr-Universität Bochum, GERMANY

Session reference: 6CV.6.20